I just tried with the official signal client, and I don't think there's a way to do it without transferring the account to another device. The second app must remain open while the first app scans the code, so while it's possible in a private space, I think profiles are too isolated to run both at once. I'd be happy to be proven otherwise, but from what I can tell, it's not possible on one device alone. I'd imagine Molly is the same.
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